Selective CO2-Hydrogenation using a membrane reactor

Mohammad Sadegh Salehi (Corresponding author), Maryam Askarishahi, Fausto Gallucci, Hamid Reza Godini (Corresponding author)

Onderzoeksoutput: Bijdrage aan tijdschriftTijdschriftartikelAcademicpeer review

Samenvatting

We present a novel membrane reactor (MR) concept for CO2 -hydrogenation to methanol application, in which CO2 is supplied from a CO2 -rich gas stream via a membrane and is distributed along the catalytic packed bed, where it reacts with hydrogen over a CuO-ZnO/Al2O3 catalyst to produce methanol. The performance of the reactor was investigated using a set of two-fluid model simulations. The simulation results showed that the fine distribution of CO2 improved the selectivity of methanol production by a value of 6 % for the studied range of the operating conditions.

Originele taal-2Engels
Artikelnummer108264
Aantal pagina's10
TijdschriftChemical Engineering and Processing - Process Intensification
Volume160
DOI's
StatusGepubliceerd - mrt 2021

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