Packed bed Ca-Cu looping process integrated with a natural gas, combined cycle for low emission power production

M. Martini; I. Martinez; F. Gallucci; M.C. Romano; P. Chiesa; M. van Sint Annaland

doi:10.1016/j.egypro.2017.03.1153

Packed bed Ca-Cu looping process integrated with a natural gas, combined cycle for low emission power production

M. Martini, I. Martinez, F. Gallucci, M.C. Romano, P. Chiesa, M. van Sint Annaland

Chemical Process Intensification

Onderzoeksoutput: Bijdrage aan tijdschrift › Tijdschriftartikel › Academic › peer review

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This work investigates the full process design of a natural gas combined cycle integrated with a packed-bed reactor system where a hydrogen rich gas is produced with inherent CO2 capture based of the CaO/CaCO3 and Cu/CuO chemical loops. The different stages of this Ca-Cu process were modelled with a dynamic 1D pseudo-homogeneous model, proposing a novel reactor configuration allowing to achieve carbon capture efficiency close to 90%. Process simulations of the whole power plant resulted in electric efficiencies of around 48%LHV and SPECCA of 4.7 MJ/kgCO2.

Originele taal-2	Engels
Pagina's (van-tot)	104-112
Aantal pagina's	9
Tijdschrift	Energy Procedia
Volume	114
DOI's	https://doi.org/10.1016/j.egypro.2017.03.1153
Status	Gepubliceerd - 2017
Evenement	13th International Conference on Greenhouse Gas Control Technologies, (GHGT-13) - Lausanne, Zwitserland Duur: 14 nov 2016 → 18 nov 2016 http://www.ghgt.info/ghgt-13/ghgt-13-programme

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10.1016/j.egypro.2017.03.1153

Publishers versionDefinitieve gepubliceerde versie, 226 KBLicentie: CC BY-NC-ND

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Citeer dit

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title = "Packed bed Ca-Cu looping process integrated with a natural gas, combined cycle for low emission power production",

abstract = "This work investigates the full process design of a natural gas combined cycle integrated with a packed-bed reactor system where a hydrogen rich gas is produced with inherent CO2 capture based of the CaO/CaCO3 and Cu/CuO chemical loops. The different stages of this Ca-Cu process were modelled with a dynamic 1D pseudo-homogeneous model, proposing a novel reactor configuration allowing to achieve carbon capture efficiency close to 90%. Process simulations of the whole power plant resulted in electric efficiencies of around 48%LHV and SPECCA of 4.7 MJ/kgCO2.",

keywords = "CO capture, Chemical looping, Modeling, Power production, Sorption enhanced reforming",

author = "M. Martini and I. Martinez and F. Gallucci and M.C. Romano and P. Chiesa and {van Sint Annaland}, M.",

year = "2017",

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AU - Martini, M.

AU - Martinez, I.

AU - Gallucci, F.

AU - Romano, M.C.

AU - Chiesa, P.

AU - van Sint Annaland, M.

PY - 2017

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AB - This work investigates the full process design of a natural gas combined cycle integrated with a packed-bed reactor system where a hydrogen rich gas is produced with inherent CO2 capture based of the CaO/CaCO3 and Cu/CuO chemical loops. The different stages of this Ca-Cu process were modelled with a dynamic 1D pseudo-homogeneous model, proposing a novel reactor configuration allowing to achieve carbon capture efficiency close to 90%. Process simulations of the whole power plant resulted in electric efficiencies of around 48%LHV and SPECCA of 4.7 MJ/kgCO2.

KW - CO capture

KW - Chemical looping

KW - Modeling

KW - Power production

KW - Sorption enhanced reforming

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JF - Energy Procedia

SN - 1876-6102

T2 - 13th International Conference on Greenhouse Gas Control Technologies, (GHGT-13)

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