Nitric oxide formation in H2/CO syngas non-premixed jet flames

K.K.J. Ranga Dinesh, E.S. Richardson, J.A. van Oijen, K.H. Luo, X. Jiang

Onderzoeksoutput: Hoofdstuk in Boek/Rapport/CongresprocedureConferentiebijdrageAcademicpeer review

Samenvatting

Direct numerical simulations (DNS) of high hydrogen content (HHC) syngas nonpremixed jet flames have been carried out to study the nitric oxide (NO) formation. The detailed chemistry employed is the GRI 3.0 updated with the influence of the NCN radical chemistry using flamelet generated manifolds (FGM). Preferential diffusion effects have been considered via FGM tabulation and the progress variable transport equation. The results indicate a strong correlation between the flame temperature and NO concentration for pure H2 flame, in which NO formation is characterised by the thermal and NNH mechanisms. The results also indicate a rapid decrease of maximum NO values in the syngas mixtures due to lower temperatures associated with the CO-dilution into H2, thereby increasing the contribution of the prompt-NO mechanism via CH radicals.

Originele taal-2Engels
TitelThe 12th International Conference on Combustion & Energy Utilisation, 12ICCEU 
Plaats van productieAmsterdam
UitgeverijElsevier
Pagina's5-8
Aantal pagina's4
DOI's
StatusGepubliceerd - 2015
Evenement23rd International Conference on the Application of Accelerators in Research and Industry, CAARI 2014 - San Antonio, Verenigde Staten van Amerika
Duur: 25 mei 201430 mei 2014

Publicatie series

NaamEnergy Procedia
Volume66

Congres

Congres23rd International Conference on the Application of Accelerators in Research and Industry, CAARI 2014
Land/RegioVerenigde Staten van Amerika
StadSan Antonio
Periode25/05/1430/05/14

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