Milliwatt terahertz harmonic generation from topological insulator metamaterials

Klaas-Jan Tielrooij (Corresponding author), Alessandro Principi, David Saleta Reig, Alexander Block, Sebin Varghese, Steffen Schreyeck, Karl Brunner, Grzegorz Karczewski, Igor Ilyakov, Oleksiy Ponomaryov, Thales V.A.G. de Oliveira, Min Chen, Jan-Christoph Deinert, Carmen Gomez Carbonell, Sergio O. Valenzuela, Laurens W. Molenkamp, Tobias Kiessling, Georgy V. Astakhov (Corresponding author), Sergey Kovalev (Corresponding author)

Onderzoeksoutput: Bijdrage aan tijdschriftTijdschriftartikelAcademicpeer review

11 Citaten (Scopus)
33 Downloads (Pure)


Achieving efficient, high-power harmonic generation in the terahertz spectral domain has technological applications, for example, in sixth generation (6G) communication networks. Massless Dirac fermions possess extremely large terahertz nonlinear susceptibilities and harmonic conversion efficiencies. However, the observed maximum generated harmonic power is limited, because of saturation effects at increasing incident powers, as shown recently for graphene. Here, we demonstrate room-temperature terahertz harmonic generation in a Bi2Se3 topological insulator and topological-insulator-grating metamaterial structures with surface-selective terahertz field enhancement. We obtain a third-harmonic power approaching the milliwatt range for an incident power of 75 mW—an improvement by two orders of magnitude compared to a benchmarked graphene sample. We establish a framework in which this exceptional performance is the result of thermodynamic harmonic generation by the massless topological surface states, benefiting from ultrafast dissipation of electronic heat via surface-bulk Coulomb interactions. These results are an important step towards on-chip terahertz (opto)electronic applications.

Originele taal-2Engels
Aantal pagina's8
TijdschriftLight: Science and Applications
StatusGepubliceerd - 1 nov. 2022

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