Metal–Organic Frameworks and Water: ‘From Old Enemies to Friends’?

Georges Mouchaham; Frédéric S. Cui; Farid Nouar; Vanessa Pimenta; Jong San Chang; Christian Serre

doi:10.1016/j.trechm.2020.09.004

Metal–Organic Frameworks and Water: ‘From Old Enemies to Friends’?

Georges Mouchaham (Corresponding author), Frédéric S. Cui, Farid Nouar, Vanessa Pimenta, Jong San Chang, Christian Serre

Onderzoeksoutput: Bijdrage aan tijdschrift › Artikel recenseren › peer review

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Since their discovery a few decades ago, metal–organic frameworks (MOFs) have suffered from poor hydrolytic stability. Since then, significant effort has been devoted to design robust MOFs, including their utilization for water-related applications to overcome relevant societal challenges. This short review provides guidelines on the key parameters that drive the assembly of hydrothermally stable MOFs together with the most relevant physicochemical features needed in their water-related applications. It also highlights some of the recent advances in MOF-water applications (based on water sorption or mediation and separation in the presence of water) as well as the most critical challenges to overcome.

Originele taal-2	Engels
Pagina's (van-tot)	990-1003
Aantal pagina's	14
Tijdschrift	Trends in Chemistry
Volume	2
Nummer van het tijdschrift	11
DOI's	https://doi.org/10.1016/j.trechm.2020.09.004
Status	Gepubliceerd - nov. 2020

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© 2020 Elsevier Inc.

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G.M., F.N., and C.S. acknowledge the CNRS, ENS, ESPCI, and PSL University for financial support. F.S.C. acknowledges funding from the EU’s H2020 Programme under MSCA grant agreement no. 754462. G.M. F.N. and C.S. acknowledge the CNRS, ENS, ESPCI, and PSL University for financial support. F.S.C. acknowledges funding from the EU's H2020 Programme under MSCA grant agreement no. 754462.

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title = "Metal–Organic Frameworks and Water: {\textquoteleft}From Old Enemies to Friends{\textquoteright}?",

abstract = "Since their discovery a few decades ago, metal–organic frameworks (MOFs) have suffered from poor hydrolytic stability. Since then, significant effort has been devoted to design robust MOFs, including their utilization for water-related applications to overcome relevant societal challenges. This short review provides guidelines on the key parameters that drive the assembly of hydrothermally stable MOFs together with the most relevant physicochemical features needed in their water-related applications. It also highlights some of the recent advances in MOF-water applications (based on water sorption or mediation and separation in the presence of water) as well as the most critical challenges to overcome.",

keywords = "hydrolytic stability, metal–organic framework, MOF, sorption, water-based applications",

author = "Georges Mouchaham and Cui, {Fr{\'e}d{\'e}ric S.} and Farid Nouar and Vanessa Pimenta and Chang, {Jong San} and Christian Serre",

note = "Funding Information: G.M., F.N., and C.S. acknowledge the CNRS, ENS, ESPCI, and PSL University for financial support. F.S.C. acknowledges funding from the EU{\textquoteright}s H2020 Programme under MSCA grant agreement no. 754462. ",

year = "2020",

month = nov,

doi = "10.1016/j.trechm.2020.09.004",

language = "English",

volume = "2",

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T2 - ‘From Old Enemies to Friends’?

AU - Mouchaham, Georges

AU - Cui, Frédéric S.

AU - Nouar, Farid

AU - Pimenta, Vanessa

AU - Chang, Jong San

AU - Serre, Christian

N1 - Funding Information: G.M., F.N., and C.S. acknowledge the CNRS, ENS, ESPCI, and PSL University for financial support. F.S.C. acknowledges funding from the EU’s H2020 Programme under MSCA grant agreement no. 754462.

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N2 - Since their discovery a few decades ago, metal–organic frameworks (MOFs) have suffered from poor hydrolytic stability. Since then, significant effort has been devoted to design robust MOFs, including their utilization for water-related applications to overcome relevant societal challenges. This short review provides guidelines on the key parameters that drive the assembly of hydrothermally stable MOFs together with the most relevant physicochemical features needed in their water-related applications. It also highlights some of the recent advances in MOF-water applications (based on water sorption or mediation and separation in the presence of water) as well as the most critical challenges to overcome.

AB - Since their discovery a few decades ago, metal–organic frameworks (MOFs) have suffered from poor hydrolytic stability. Since then, significant effort has been devoted to design robust MOFs, including their utilization for water-related applications to overcome relevant societal challenges. This short review provides guidelines on the key parameters that drive the assembly of hydrothermally stable MOFs together with the most relevant physicochemical features needed in their water-related applications. It also highlights some of the recent advances in MOF-water applications (based on water sorption or mediation and separation in the presence of water) as well as the most critical challenges to overcome.

KW - hydrolytic stability

KW - metal–organic framework

KW - MOF

KW - sorption

KW - water-based applications

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U2 - 10.1016/j.trechm.2020.09.004

DO - 10.1016/j.trechm.2020.09.004

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Metal–Organic Frameworks and Water: ‘From Old Enemies to Friends’?

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