Imaging of n-hexane in zeolites by positron emission profiling (PEP)

R.A. van Santen; B.G. Anderson; R.H. Cunningham; A.V.G. Mangnus; J. van Grondelle; L.J. IJzendoorn, van

doi:10.1016/S0167-2991(96)80290-4

Imaging of n-hexane in zeolites by positron emission profiling (PEP)

R.A. van Santen, B.G. Anderson, R.H. Cunningham, A.V.G. Mangnus, J. van Grondelle, L.J. IJzendoorn, van

Onderzoeksoutput: Hoofdstuk in Boek/Rapport/Congresprocedure › Conferentiebijdrage › Academic

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Samenvatting

Positron Emission Profiling (PEP) has been used for in-situ measurement of the surface coverage of H-mordenite by n-hexane, as a function of hexane partial pressure, at the elevated temperatures typically used for hydroisomerization by monitoring the retention time of an injected radio-labelled pulse of n-hexane. The labelled molecules ((CH3C5H11)-C-11) were produced via a two-step alkene homologation reaction in which C-11, produced using a cyclotron, was added to 1-pentene. The PEP method described is similar to the ''tracer pulse technique'' however it has the significant advantage of in-situ imaging of the pulse

Originele taal-2	Engels
Titel	11th international congress on catalysis-40th anniversary; proceedings of the11th ICC, Baltimore, MD, USA 30-06-1996 - 5-07-1996. Part B
Redacteuren	J.W. Hightower, W.N. Delgass, E. Iglesia, A.T. Bell
Plaats van productie	Amsterdam
Uitgeverij	Elsevier
Pagina's	791-800
ISBN van geprinte versie	0-444-81947-9
DOI's	https://doi.org/10.1016/S0167-2991(96)80290-4
Status	Gepubliceerd - 1996
Evenement	11th International Congress on Catalysis (ICC 1996) - Baltimore, MD, Verenigde Staten van Amerika Duur: 30 jun 1996 → 5 jul 1996 Congresnummer: 11

Publicatie series

Naam	Studies in Surface Science and Catalysis
Nummer	Part B
Volume	101
ISSN van geprinte versie	0167-2991

Congres

Congres	11th International Congress on Catalysis (ICC 1996)
Verkorte titel	ICC 1996
Land	Verenigde Staten van Amerika
Stad	Baltimore, MD
Periode	30/06/96 → 5/07/96

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10.1016/S0167-2991(96)80290-4

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van Santen, R. A., Anderson, B. G., Cunningham, R. H., Mangnus, A. V. G., van Grondelle, J., & IJzendoorn, van, L. J. (1996). Imaging of n-hexane in zeolites by positron emission profiling (PEP). In J. W. Hightower, W. N. Delgass, E. Iglesia, & A. T. Bell (editors), 11th international congress on catalysis-40th anniversary; proceedings of the11th ICC, Baltimore, MD, USA 30-06-1996 - 5-07-1996. Part B (blz. 791-800). (Studies in Surface Science and Catalysis; Vol. 101, Nr. Part B). Amsterdam: Elsevier. https://doi.org/10.1016/S0167-2991(96)80290-4

van Santen, R.A. ; Anderson, B.G. ; Cunningham, R.H. ; Mangnus, A.V.G. ; van Grondelle, J. ; IJzendoorn, van, L.J. / Imaging of n-hexane in zeolites by positron emission profiling (PEP). 11th international congress on catalysis-40th anniversary; proceedings of the11th ICC, Baltimore, MD, USA 30-06-1996 - 5-07-1996. Part B. redacteur / J.W. Hightower ; W.N. Delgass ; E. Iglesia ; A.T. Bell. Amsterdam : Elsevier, 1996. blz. 791-800 (Studies in Surface Science and Catalysis; Part B).

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title = "Imaging of n-hexane in zeolites by positron emission profiling (PEP)",

abstract = "Positron Emission Profiling (PEP) has been used for in-situ measurement of the surface coverage of H-mordenite by n-hexane, as a function of hexane partial pressure, at the elevated temperatures typically used for hydroisomerization by monitoring the retention time of an injected radio-labelled pulse of n-hexane. The labelled molecules ((CH3C5H11)-C-11) were produced via a two-step alkene homologation reaction in which C-11, produced using a cyclotron, was added to 1-pentene. The PEP method described is similar to the ''tracer pulse technique'' however it has the significant advantage of in-situ imaging of the pulse",

author = "{van Santen}, R.A. and B.G. Anderson and R.H. Cunningham and A.V.G. Mangnus and {van Grondelle}, J. and {IJzendoorn, van}, L.J.",

year = "1996",

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van Santen, RA, Anderson, BG, Cunningham, RH, Mangnus, AVG, van Grondelle, J & IJzendoorn, van, LJ 1996, Imaging of n-hexane in zeolites by positron emission profiling (PEP). in JW Hightower, WN Delgass, E Iglesia & AT Bell (redactie), 11th international congress on catalysis-40th anniversary; proceedings of the11th ICC, Baltimore, MD, USA 30-06-1996 - 5-07-1996. Part B. Studies in Surface Science and Catalysis, nr. Part B, vol. 101, Elsevier, Amsterdam, blz. 791-800, 11th International Congress on Catalysis (ICC 1996), Baltimore, MD, Verenigde Staten van Amerika, 30/06/96. https://doi.org/10.1016/S0167-2991(96)80290-4

Imaging of n-hexane in zeolites by positron emission profiling (PEP). / van Santen, R.A.; Anderson, B.G.; Cunningham, R.H.; Mangnus, A.V.G.; van Grondelle, J.; IJzendoorn, van, L.J.

11th international congress on catalysis-40th anniversary; proceedings of the11th ICC, Baltimore, MD, USA 30-06-1996 - 5-07-1996. Part B. redactie / J.W. Hightower; W.N. Delgass; E. Iglesia; A.T. Bell. Amsterdam : Elsevier, 1996. blz. 791-800 (Studies in Surface Science and Catalysis; Vol. 101, Nr. Part B).

Onderzoeksoutput: Hoofdstuk in Boek/Rapport/Congresprocedure › Conferentiebijdrage › Academic

TY - GEN

T1 - Imaging of n-hexane in zeolites by positron emission profiling (PEP)

AU - van Santen, R.A.

AU - Anderson, B.G.

AU - Cunningham, R.H.

AU - Mangnus, A.V.G.

AU - van Grondelle, J.

AU - IJzendoorn, van, L.J.

PY - 1996

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N2 - Positron Emission Profiling (PEP) has been used for in-situ measurement of the surface coverage of H-mordenite by n-hexane, as a function of hexane partial pressure, at the elevated temperatures typically used for hydroisomerization by monitoring the retention time of an injected radio-labelled pulse of n-hexane. The labelled molecules ((CH3C5H11)-C-11) were produced via a two-step alkene homologation reaction in which C-11, produced using a cyclotron, was added to 1-pentene. The PEP method described is similar to the ''tracer pulse technique'' however it has the significant advantage of in-situ imaging of the pulse

AB - Positron Emission Profiling (PEP) has been used for in-situ measurement of the surface coverage of H-mordenite by n-hexane, as a function of hexane partial pressure, at the elevated temperatures typically used for hydroisomerization by monitoring the retention time of an injected radio-labelled pulse of n-hexane. The labelled molecules ((CH3C5H11)-C-11) were produced via a two-step alkene homologation reaction in which C-11, produced using a cyclotron, was added to 1-pentene. The PEP method described is similar to the ''tracer pulse technique'' however it has the significant advantage of in-situ imaging of the pulse

U2 - 10.1016/S0167-2991(96)80290-4

DO - 10.1016/S0167-2991(96)80290-4

M3 - Conference contribution

SN - 0-444-81947-9

T3 - Studies in Surface Science and Catalysis

SP - 791

EP - 800

BT - 11th international congress on catalysis-40th anniversary; proceedings of the11th ICC, Baltimore, MD, USA 30-06-1996 - 5-07-1996. Part B

A2 - Hightower, J.W.

A2 - Delgass, W.N.

A2 - Iglesia, E.

A2 - Bell, A.T.

PB - Elsevier

CY - Amsterdam

ER -

van Santen RA, Anderson BG, Cunningham RH, Mangnus AVG, van Grondelle J, IJzendoorn, van LJ. Imaging of n-hexane in zeolites by positron emission profiling (PEP). In Hightower JW, Delgass WN, Iglesia E, Bell AT, redacteurs, 11th international congress on catalysis-40th anniversary; proceedings of the11th ICC, Baltimore, MD, USA 30-06-1996 - 5-07-1996. Part B. Amsterdam: Elsevier. 1996. blz. 791-800. (Studies in Surface Science and Catalysis; Part B). https://doi.org/10.1016/S0167-2991(96)80290-4