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Free-standing bilayer metasurfaces in the visible

  • Ahmed Dorrah
  • , Alfonso Palmieri
  • , Joon-Suh Park
  • , Federico Capasso (Corresponding author)

Onderzoeksoutput: Bijdrage aan tijdschriftTijdschriftartikelAcademicpeer review

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Samenvatting

Multi-layered meta-optics have enabled complex wavefront shaping beyond their single layer counterpart owing to the additional design variables afforded by each plane. For instance, lossless complex amplitude modulation, generalized polarization transformations, and wide field of view are key attributes that fundamentally require multi-plane wavefront matching. Nevertheless, existing embodiments of bilayer metasurfaces have relied on configurations which suffer from Fresnel reflections, low mode confinement, or undesired resonances which compromise the intended response. Here, we introduce bilayer metasurfaces made of free-standing meta-atoms working in the visible spectrum. We demonstrate their use in wavefront shaping of linearly polarized light using pure geometric phase with diffraction efficiency of 80% — expanding previous literature on Pancharatnam-Berry phase metasurfaces which rely on circularly or elliptically polarized illumination. The fabrication relies on a two-step lithography and selective development processes which yield free standing, bilayer stacked metasurfaces, of 1200 nm total thickness. The metasurfaces comprise TiO2 nanofins with vertical sidewalls. Our work advances the nanofabrication of compound meta-optics and inspires new directions in wavefront shaping, metasurface integration, and polarization control.
Originele taal-2Engels
Artikelnummer3126
Aantal pagina's10
TijdschriftNature Communications
Volume16
DOI's
StatusGepubliceerd - 1 apr. 2025

Financiering

We thank Jaewon Oh, Aun Zaidi, Noah A. Rubin, and Kerolos M.A. Yousef from Harvard University, as well as Paulo Dainese from Corning Inc., and Jasper van der Weert from TU Eindhoven for their insightful discussions. We also acknowledge the help of staff from Harvard’s Center for Nanoscale Systems (CNS); Stephan Kraemer with the FIB process, and Mac Hathaway with the ALD process. A.H.D. acknowledges financial support from the Optica Foundation Challenge program. F.C. acknowledges financial support from the Office of Naval Research (ONR) under the MURI program, grant no. N00014-20-1-2450, and from the Air Force Office of Scientific Research (AFOSR) under grant nos FA9550-21-1-0312 and FA9550-22-1-0243. This work was performed at the Harvard University Center for Nanoscale Systems (CNS); a member of the National Nanotechnology Coordinated Infrastructure Network (NNCI), which is supported by the National Science Foundation under NSF award no. ECCS-2025158. The simulation work was in part performed using Tidy3D software from Flexcompute.

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