Effect of anisotropic scattering for rotational collisions on electron transport parameters in CO

Luca Vialetto (Corresponding author), Adel Ben Moussa, Jan van Dijk, Savino Longo, Paola Diomede, Vasco Guerra, Luis Lemos Alves

Onderzoeksoutput: Bijdrage aan tijdschriftTijdschriftartikelAcademicpeer review

Samenvatting

The role of anisotropic scattering in rotational collisions of electrons with CO molecules is investigated numerically with Monte Carlo (MC) simulations and with calculations using the Lisbon KInetics two-term Boltzmann solver (LoKI- B). The study adopts integral cross sections taken from the IST-Lisbon database of LXCat or extracted from Biagi’s code Magboltz v11.10. Different angular scattering models for rotational collisions are implemented and compared in MC simulations, and a novel anisotropic scattering model is derived from the dipole-Born differential cross sections, to describe the strongly forward-peaked nature of rotational collisions. This model is also implemented in LoKI-B, to describe the anisotropic inelastic/superelastic scattering in dipole rotational collisions, using coherent expressions for the corresponding integral and momentum transfer cross sections. The comparison between MC and LoKI-B results shows that the calculation of swarm parameters is more influenced by the choice of the angular scattering model than the adoption of the two-term approximation, yielding deviations up to 50% in the reduced mobility for different angular distributions. The consequences in the swarm derivation of cross sections are also discussed. Finally, it is shown that inclusion of electric-quadrupole interactions, usually neglected in electron swarm studies, can improve the agreement between numerical results and measurements.
Originele taal-2 Engels 075001 20 Plasma Sources Science and Technology 30 7 https://doi.org/10.1088/1361-6595/ac0a4d Gepubliceerd - 1 jul 2021

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