Many gas-liquid-solid contactors, such as trickle bed and bubble slurry columns, suffer from heat and mass transfer limitations. To overcome these limitations, new micro-structured bubble column reactor is proposed. In this reactor, a catalyst coated wire mesh is introduced in a bubble column to cut the bubbles and enhance the interface dynamics. In this work, the effect of the simplest form of a wire mesh, i.e. a single wire, on a single bubble is studied experimentally and using Direct Numerical Simulations. The combined Volume of Fluid and Immersed Boundary method shows a good agreement with the experimentally obtained bubble sizes after cutting, bubble shapes, trajectory and bubble rise velocities. Only small differences are found in the bubble rise velocity in close proximity of the wire. Various effects were determined both experimentally and numerically: the effects of Eötvös number, Morton number, bubble rise velocity, wire diameter and the obliqueness of the bubble wire interactions. From the results, it can be concluded that the main influences on the bubble cutting are the Eötvös number, the wire diameter and the obliqueness of the interaction. However, a quantitative closure for the bubble cutting using single wires could not be obtained.
|Tijdschrift||Chemical Engineering Science|
|Status||Gepubliceerd - 10 jan 2017|
|Evenement||12th International Conference on Gas-Liquid & Gas-Liquid-Solid Reactor Engineering (GLS 12), June 28-July 1, 2015, New York, NY, USA - New York, NY, Verenigde Staten van Amerika|
Duur: 28 jun 2015 → 1 jul 2015