CO2 hydrogenation in a dielectric barrier discharge plasma revealed

C. De Bie, J. van Dijk, A. Bogaerts

Onderzoeksoutput: Bijdrage aan tijdschriftTijdschriftartikelAcademicpeer review

18 Citaten (Scopus)

Samenvatting

The hydrogenation of carbon dioxide in a dielectric barrier discharge plasma is studied with a one-dimensional fluid model. The spatially averaged densities of the most important end products formed in the CO2/H2 mixture are determined as a function of the initial gas mixing ratio. CO and H2O are found to be present at the highest densities and to a lower content also CH4, C2H6, CH2O, CH3OH, O2, and some other higher hydrocarbons and oxygenates. The main underlying reaction pathways for the conversion of the inlet gases and the formation of CO, CH4, CH2O, and CH3OH are pointed out for various gas mixing ratios. The CO2 conversion and the production of value added products is found to be quite low, also in comparison to a CO2/CH4 mixture, and this can be explained by the model.
Originele taal-2Engels
Pagina's (van-tot)25210-25224
Aantal pagina's25
TijdschriftJournal of Physical Chemistry C
DOI's
StatusGepubliceerd - 19 okt 2016

    Vingerafdruk

Citeer dit