Bipolaron mechanism for organic magnetoresistance

P.A. Bobbert, T.D. Nguyen, F.W.A. Oost, van, B. Koopmans, M. Wohlgenannt

Onderzoeksoutput: Bijdrage aan tijdschriftTijdschriftartikelAcademicpeer review

372 Citaties (Scopus)

Uittreksel

We present a mechanism for the recently discovered magnetoresistance in disordered ?-conjugated materials, based on hopping of polarons and bipolaron formation, in the presence of the random hyperfine fields of the hydrogen nuclei and an external magnetic field. Within a simple model we describe the magnetic field dependence of the bipolaron density. MonteCarlo simulations including on-site and longer-range Coulomb repulsion show how this leads to positive and negative magnetoresistance. Depending on the branching ratio between bipolaron formation or dissociation and hopping rates, two different line shapes in excellent agreement with experiment are obtained.
TaalEngels
Artikelnummer216801
Pagina's216801-1/4
Aantal pagina's4
TijdschriftPhysical Review Letters
Volume99
Nummer van het tijdschrift21
DOI's
StatusGepubliceerd - 2007

Vingerafdruk

polarons
magnetic fields
line shape
dissociation
nuclei
hydrogen
simulation

Citeer dit

Bobbert, P. A., Nguyen, T. D., Oost, van, F. W. A., Koopmans, B., & Wohlgenannt, M. (2007). Bipolaron mechanism for organic magnetoresistance. Physical Review Letters, 99(21), 216801-1/4. [216801]. DOI: 10.1103/PhysRevLett.99.216801
Bobbert, P.A. ; Nguyen, T.D. ; Oost, van, F.W.A. ; Koopmans, B. ; Wohlgenannt, M./ Bipolaron mechanism for organic magnetoresistance. In: Physical Review Letters. 2007 ; Vol. 99, Nr. 21. blz. 216801-1/4
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Bobbert, PA, Nguyen, TD, Oost, van, FWA, Koopmans, B & Wohlgenannt, M 2007, 'Bipolaron mechanism for organic magnetoresistance' Physical Review Letters, vol. 99, nr. 21, 216801, blz. 216801-1/4. DOI: 10.1103/PhysRevLett.99.216801

Bipolaron mechanism for organic magnetoresistance. / Bobbert, P.A.; Nguyen, T.D.; Oost, van, F.W.A.; Koopmans, B.; Wohlgenannt, M.

In: Physical Review Letters, Vol. 99, Nr. 21, 216801, 2007, blz. 216801-1/4.

Onderzoeksoutput: Bijdrage aan tijdschriftTijdschriftartikelAcademicpeer review

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Bobbert PA, Nguyen TD, Oost, van FWA, Koopmans B, Wohlgenannt M. Bipolaron mechanism for organic magnetoresistance. Physical Review Letters. 2007;99(21):216801-1/4. 216801. Beschikbaar vanaf, DOI: 10.1103/PhysRevLett.99.216801