A novel catalyst-sorbent system for an efficient H2 production with in-situ CO2 capture

M.H. Halabi; M.H.J.M. Croon, de; J. Schaaf, van der; P.D. Cobden; J.C. Schouten

doi:10.1016/j.ijhydene.2011.12.025

A novel catalyst-sorbent system for an efficient H2 production with in-situ CO2 capture

M.H. Halabi, M.H.J.M. Croon, de, J. Schaaf, van der, P.D. Cobden, J.C. Schouten

Chemical Reactor Engineering

Onderzoeksoutput: Bijdrage aan tijdschrift › Tijdschriftartikel › Academic › peer review

26 Citaten (Scopus)

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This paper presents an experimental investigation for an improved process of sorption-enhanced steam reforming of methane in an admixture fixed bed reactor. A highly active Rh/CeaZr1-aO2 catalyst and K2CO3-promoted hydrotalcite are utilized as novel catalyst/sorbent materials for an efficient H2 production with in situ CO2 capture at low temperature (450–500 °C). The process performance is demonstrated in response to temperature (400–500 °C), pressure (1.5–6.0 bar), and steam/carbon ratio (3–6). Thus, direct production of high H2 purity and fuel conversion >99% is achieved with low level of carbon oxides impurities (

Originele taal-2	Engels
Pagina's (van-tot)	4987-4996
Aantal pagina's	9
Tijdschrift	International Journal of Hydrogen Energy
Volume	37
Nummer van het tijdschrift	6
DOI's	https://doi.org/10.1016/j.ijhydene.2011.12.025
Status	Gepubliceerd - 2012

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title = "A novel catalyst-sorbent system for an efficient H2 production with in-situ CO2 capture",

abstract = "This paper presents an experimental investigation for an improved process of sorption-enhanced steam reforming of methane in an admixture fixed bed reactor. A highly active Rh/CeaZr1-aO2 catalyst and K2CO3-promoted hydrotalcite are utilized as novel catalyst/sorbent materials for an efficient H2 production with in situ CO2 capture at low temperature (450–500 °C). The process performance is demonstrated in response to temperature (400–500 °C), pressure (1.5–6.0 bar), and steam/carbon ratio (3–6). Thus, direct production of high H2 purity and fuel conversion >99% is achieved with low level of carbon oxides impurities (",

author = "M.H. Halabi and {Croon, de}, M.H.J.M. and {Schaaf, van der}, J. and P.D. Cobden and J.C. Schouten",

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AU - Cobden, P.D.

AU - Schouten, J.C.

PY - 2012

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AB - This paper presents an experimental investigation for an improved process of sorption-enhanced steam reforming of methane in an admixture fixed bed reactor. A highly active Rh/CeaZr1-aO2 catalyst and K2CO3-promoted hydrotalcite are utilized as novel catalyst/sorbent materials for an efficient H2 production with in situ CO2 capture at low temperature (450–500 °C). The process performance is demonstrated in response to temperature (400–500 °C), pressure (1.5–6.0 bar), and steam/carbon ratio (3–6). Thus, direct production of high H2 purity and fuel conversion >99% is achieved with low level of carbon oxides impurities (

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JO - International Journal of Hydrogen Energy

JF - International Journal of Hydrogen Energy

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ER -

A novel catalyst-sorbent system for an efficient H2 production with in-situ CO2 capture

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