A chaotic self-oscillating sunlight driven polymer actuator

K. Kumar, Chr. Knie, D. Bleger, M.A. Peletier, H.B. Friedrich, S. Hecht, D.J. Broer, M.G. Debije, A.P.H.J. Schenning

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Uittreksel

Nature provides much inspiration for the design of materials capable of motion upon exposure to external stimuli, and many examples of such active systems have been created in the laboratory. However, to achieve continuous motion driven by an unchanging, constant stimulus has proven extremely challenging. Here we describe a liquid crystalline polymer film doped with a visible light responsive fluorinated azobenzene capable of continuous chaotic oscillatory motion when exposed to ambient sunlight in air. The presence of simultaneous illumination by blue and green light is necessary for the oscillating behavior to occur, suggesting that the dynamics of continuous forward and backward switching are causing the observed effect. Our work constitutes an important step towards the realization of autonomous, persistently self-propelling machines and self-cleaning surfaces powered by sunlight.
Originele taal-2Engels
Artikelnummer11975
Aantal pagina's8
TijdschriftNature Communications
Volume7
DOI's
StatusGepubliceerd - 4 jul 2016

Vingerafdruk

Surface cleaning
Methyl Green
Sunlight
Liquid crystal polymers
sunlight
Polymer films
Polymers
Actuators
Lighting
actuators
stimuli
polymers
Air
inspiration
cleaning
illumination
Light
air
liquids
azobenzene

Citeer dit

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abstract = "Nature provides much inspiration for the design of materials capable of motion upon exposure to external stimuli, and many examples of such active systems have been created in the laboratory. However, to achieve continuous motion driven by an unchanging, constant stimulus has proven extremely challenging. Here we describe a liquid crystalline polymer film doped with a visible light responsive fluorinated azobenzene capable of continuous chaotic oscillatory motion when exposed to ambient sunlight in air. The presence of simultaneous illumination by blue and green light is necessary for the oscillating behavior to occur, suggesting that the dynamics of continuous forward and backward switching are causing the observed effect. Our work constitutes an important step towards the realization of autonomous, persistently self-propelling machines and self-cleaning surfaces powered by sunlight.",
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A chaotic self-oscillating sunlight driven polymer actuator. / Kumar, K.; Knie, Chr.; Bleger, D.; Peletier, M.A.; Friedrich, H.B.; Hecht, S.; Broer, D.J.; Debije, M.G.; Schenning, A.P.H.J.

In: Nature Communications, Vol. 7, 11975, 04.07.2016.

Onderzoeksoutput: Bijdrage aan tijdschriftTijdschriftartikelAcademicpeer review

TY - JOUR

T1 - A chaotic self-oscillating sunlight driven polymer actuator

AU - Kumar, K.

AU - Knie, Chr.

AU - Bleger, D.

AU - Peletier, M.A.

AU - Friedrich, H.B.

AU - Hecht, S.

AU - Broer, D.J.

AU - Debije, M.G.

AU - Schenning, A.P.H.J.

PY - 2016/7/4

Y1 - 2016/7/4

N2 - Nature provides much inspiration for the design of materials capable of motion upon exposure to external stimuli, and many examples of such active systems have been created in the laboratory. However, to achieve continuous motion driven by an unchanging, constant stimulus has proven extremely challenging. Here we describe a liquid crystalline polymer film doped with a visible light responsive fluorinated azobenzene capable of continuous chaotic oscillatory motion when exposed to ambient sunlight in air. The presence of simultaneous illumination by blue and green light is necessary for the oscillating behavior to occur, suggesting that the dynamics of continuous forward and backward switching are causing the observed effect. Our work constitutes an important step towards the realization of autonomous, persistently self-propelling machines and self-cleaning surfaces powered by sunlight.

AB - Nature provides much inspiration for the design of materials capable of motion upon exposure to external stimuli, and many examples of such active systems have been created in the laboratory. However, to achieve continuous motion driven by an unchanging, constant stimulus has proven extremely challenging. Here we describe a liquid crystalline polymer film doped with a visible light responsive fluorinated azobenzene capable of continuous chaotic oscillatory motion when exposed to ambient sunlight in air. The presence of simultaneous illumination by blue and green light is necessary for the oscillating behavior to occur, suggesting that the dynamics of continuous forward and backward switching are causing the observed effect. Our work constitutes an important step towards the realization of autonomous, persistently self-propelling machines and self-cleaning surfaces powered by sunlight.

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DO - 10.1038/ncomms11975

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