Thieno[3,2-b]thiophene-diketopyrrolopyrrole containing polymers for high-performance Organic Field-Effect Transistors and Organic Photovoltaic devices

H. Bronstein; Zhuoying Chen; R.S. Ashraf; Weimin Zhang; Junping Du; J.R. Durrant; P.S. Tuladhar; K. Song; S.E. Watkins; Y.H. Geerts; M.M. Wienk; R.A.J. Janssen; T.D. Anthopoulos; H. Sirringhaus; M. Heeney; I. McCulloch

doi:10.1021/ja110619k

Thieno[3,2-b]thiophene-diketopyrrolopyrrole containing polymers for high-performance Organic Field-Effect Transistors and Organic Photovoltaic devices

H. Bronstein
, Zhuoying Chen
, R.S. Ashraf
, Weimin Zhang
, Junping Du
, J.R. Durrant
, P.S. Tuladhar
, K. Song
, S.E. Watkins
, Y.H. Geerts
, M.M. Wienk
, R.A.J. Janssen
, T.D. Anthopoulos
, H. Sirringhaus
, M. Heeney
, I. McCulloch

Research output: Contribution to journal › Article › Academic › peer-review

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Abstract

We report the synthesis and polymerization of a novel thieno[3,2-b]thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm2 V-1 s-1, which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC71BM gave a power conversion efficiency of 5.4%.

Original language	English
Pages (from-to)	3272-3275
Number of pages	4
Journal	Journal of the American Chemical Society
Volume	133
Issue number	10
DOIs	https://doi.org/10.1021/ja110619k
Publication status	Published - 2011

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Bronstein, H., Chen, Z., Ashraf, R. S., Zhang, W., Du, J., Durrant, J. R., Tuladhar, P. S., Song, K., Watkins, S. E., Geerts, Y. H., Wienk, M. M., Janssen, R. A. J., Anthopoulos, T. D., Sirringhaus, H., Heeney, M., & McCulloch, I. (2011). Thieno[3,2-b]thiophene-diketopyrrolopyrrole containing polymers for high-performance Organic Field-Effect Transistors and Organic Photovoltaic devices. Journal of the American Chemical Society, 133(10), 3272-3275. https://doi.org/10.1021/ja110619k

@article{a8982b862a1a4d4b99b89ab791a4ba46,

title = "Thieno[3,2-b]thiophene-diketopyrrolopyrrole containing polymers for high-performance Organic Field-Effect Transistors and Organic Photovoltaic devices",

abstract = "We report the synthesis and polymerization of a novel thieno[3,2-b]thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm2 V-1 s-1, which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC71BM gave a power conversion efficiency of 5.4\%.",

author = "H. Bronstein and Zhuoying Chen and R.S. Ashraf and Weimin Zhang and Junping Du and J.R. Durrant and P.S. Tuladhar and K. Song and S.E. Watkins and Y.H. Geerts and M.M. Wienk and R.A.J. Janssen and T.D. Anthopoulos and H. Sirringhaus and M. Heeney and I. McCulloch",

year = "2011",

doi = "10.1021/ja110619k",

language = "English",

volume = "133",

pages = "3272--3275",

journal = "Journal of the American Chemical Society",

issn = "0002-7863",

publisher = "American Chemical Society",

number = "10",

}

Bronstein, H, Chen, Z, Ashraf, RS, Zhang, W, Du, J, Durrant, JR, Tuladhar, PS, Song, K, Watkins, SE, Geerts, YH, Wienk, MM , Janssen, RAJ, Anthopoulos, TD, Sirringhaus, H, Heeney, M & McCulloch, I 2011, 'Thieno[3,2-b]thiophene-diketopyrrolopyrrole containing polymers for high-performance Organic Field-Effect Transistors and Organic Photovoltaic devices', Journal of the American Chemical Society, vol. 133, no. 10, pp. 3272-3275. https://doi.org/10.1021/ja110619k

TY - JOUR

T1 - Thieno[3,2-b]thiophene-diketopyrrolopyrrole containing polymers for high-performance Organic Field-Effect Transistors and Organic Photovoltaic devices

AU - Bronstein, H.

AU - Chen, Zhuoying

AU - Ashraf, R.S.

AU - Zhang, Weimin

AU - Du, Junping

AU - Durrant, J.R.

AU - Tuladhar, P.S.

AU - Song, K.

AU - Watkins, S.E.

AU - Geerts, Y.H.

AU - Wienk, M.M.

AU - Janssen, R.A.J.

AU - Anthopoulos, T.D.

AU - Sirringhaus, H.

AU - Heeney, M.

AU - McCulloch, I.

PY - 2011

Y1 - 2011

N2 - We report the synthesis and polymerization of a novel thieno[3,2-b]thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm2 V-1 s-1, which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC71BM gave a power conversion efficiency of 5.4%.

AB - We report the synthesis and polymerization of a novel thieno[3,2-b]thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm2 V-1 s-1, which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC71BM gave a power conversion efficiency of 5.4%.

U2 - 10.1021/ja110619k

DO - 10.1021/ja110619k

M3 - Article

C2 - 21332134

SN - 0002-7863

VL - 133

SP - 3272

EP - 3275

JO - Journal of the American Chemical Society

JF - Journal of the American Chemical Society

IS - 10

ER -

Thieno[3,2-b]thiophene-diketopyrrolopyrrole containing polymers for high-performance Organic Field-Effect Transistors and Organic Photovoltaic devices

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