Tanks-in-series model for an auto-thermal reforming reactor with a channeled monolith

Valery A. Danilov; Gunther Kolb

doi:10.1016/j.ces.2020.116269

Tanks-in-series model for an auto-thermal reforming reactor with a channeled monolith

Valery A. Danilov, Gunther Kolb (Corresponding author)

Micro Flow Chemistry and Synthetic Methodology

Research output: Contribution to journal › Article › Academic › peer-review

3 Citations (Scopus)

Abstract

A novel tanks-in-series-reactor (TSR) model has been developed for auto-thermal reforming of hydrocarbons in a monolithic reactor carrying microchannels. The model is based on the dynamic mass and heat balance equations defined for the channel and catalyst layer. The description of chemical reactions is based on a simplified multi-step surface reaction mechanism under the assumption of the rate-determining step. The predicted steady-state concentration profiles are consistent with experimental literature data.

Original language	English
Article number	116269
Number of pages	10
Journal	Chemical Engineering Science
Volume	231
DOIs	https://doi.org/10.1016/j.ces.2020.116269
Publication status	Published - 15 Feb 2021

Keywords

Auto-thermal reforming
Dynamic
Heat transfer
Mass transfer
Mathematical modeling
Monolithic reactor

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10.1016/j.ces.2020.116269

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abstract = "A novel tanks-in-series-reactor (TSR) model has been developed for auto-thermal reforming of hydrocarbons in a monolithic reactor carrying microchannels. The model is based on the dynamic mass and heat balance equations defined for the channel and catalyst layer. The description of chemical reactions is based on a simplified multi-step surface reaction mechanism under the assumption of the rate-determining step. The predicted steady-state concentration profiles are consistent with experimental literature data.",

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AU - Kolb, Gunther

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KW - Dynamic

KW - Heat transfer

KW - Mass transfer

KW - Mathematical modeling

KW - Monolithic reactor

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JO - Chemical Engineering Science

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Tanks-in-series model for an auto-thermal reforming reactor with a channeled monolith

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Keywords

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