Tanks-in-series model for an auto-thermal reforming reactor with a channeled monolith

Valery A. Danilov, Gunther Kolb (Corresponding author)

Research output: Contribution to journalArticleAcademicpeer-review

Abstract

A novel tanks-in-series-reactor (TSR) model has been developed for auto-thermal reforming of hydrocarbons in a monolithic reactor carrying microchannels. The model is based on the dynamic mass and heat balance equations defined for the channel and catalyst layer. The description of chemical reactions is based on a simplified multi-step surface reaction mechanism under the assumption of the rate-determining step. The predicted steady-state concentration profiles are consistent with experimental literature data.

Original languageEnglish
Article number116269
Number of pages10
JournalChemical Engineering Science
Volume231
DOIs
Publication statusAccepted/In press - 5 Nov 2020

Keywords

  • Auto-thermal reforming
  • Dynamic
  • Heat transfer
  • Mass transfer
  • Mathematical modeling
  • Monolithic reactor

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