Systematics across the UTX series (T = Ru, Co, Ni; X = Al,Ga, Sn) of high-field and low-temperature properties of non-ferromagnetic compounds

V. Sechovsky, L. Havela, F.R. Boer, de, J.J.M. Franse, P.A. Veenhuizen, J. Sebek, J. Stehno, A.V. Andreev

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Abstract

Results are presented of magnetic and specific-heat studies performed on some equiatomic compounds of the series UTX with a special emphasis on non-ferromagnetic UNiAl, UCoAl, URuA1 and URuGa. The occurrence of magnetism in these compounds is attributed mainly to the 5f electrons of uranium. The systematics of the ground-state properties across the series is discussed with respect to delocalization mechanisms of the 5f electrons. The possible role of spin fluctuations in the low-temperature behaviour of UCoAl, URuAl and URuGa is indicated by magnetic measurements. The compound with the highest ¿ value, UNiAl (¿ = 167 mJ/mol K2), behaves as an itinerant antiferromagnet.
Original languageEnglish
Pages (from-to)283-293
JournalPhysica B+C
Volume142
Issue number3
DOIs
Publication statusPublished - 1986

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