Synthesis of N-doped carbon dots via a microplasma process

Xintong Ma, Sirui Li (Corresponding author), Volker Hessel, Liangliang Lin, Stefan Meskers, Fausto Gallucci

Research output: Contribution to journalArticleAcademicpeer-review

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Abstract

In this study, an effective approach was presented for the synthesis of N-doped carbon dots via a microplasma-assisted process at atmospheric pressure. The effects of operation parameters on the surface groups and photoluminescence (PL) property of carbon dots were studied in detail. Nitrogen element was successfully doped as N–H group and pyrrolic–like structure in the carbon dots. The morphology, structures, chemical compositions and photoluminescence properties of N-doped carbon dots were systematically characterized. The generated chemical species and mechanism were monitored and studied by optical emission spectroscopy. The synthesized particles owned excitation-dependent emission property with a quantum yield up to 9.90%. The plasma treatment time and operating voltage affect the carbonization degree, doping state of nitrogen and particle size, resulting in different PL behaviours. The variation of electrode sizes has slight effects on the yield of N-doped carbon dots from 0.31% to 0.42% owing to the differences in electron density.

Original languageEnglish
Article number115648
Number of pages10
JournalChemical Engineering Science
Volume220
DOIs
Publication statusPublished - 20 Jul 2020

Keywords

  • Microplasma
  • N-doped carbon dots
  • Photoluminescence

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