Abstract
We discuss an alternative to the traditional gas-phase coupling approach in order to explain synchronized global oscillations in CO oxidation on Pt(110). We use a microscopic model which includes structural Pt surface reconstruction via front propagation, and large diffusion rates for CO. The synchronization mechanism is associated with the formation of a Turing-like structure of the substrate. By using large parallel microscopic simulations we derive scaling laws which allow us to extrapolate to realistic diffusion rates, pattern size, and oscillation periods.
Original language | English |
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Article number | 031604 |
Pages (from-to) | 031604-1/4 |
Number of pages | 4 |
Journal | Physical Review E - Statistical, Nonlinear, and Soft Matter Physics |
Volume | 69 |
Issue number | 3 |
DOIs | |
Publication status | Published - 2004 |