Side-chain-functionalized polyacetylenes, 1 - Liquid crystalline and stereomutational properties

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    Abstract

    Communication: Stereospecific polymerizations of functionalized acetylenes were successfully performed using a Rh complex as the catalyst and triethylamine as a base yielding poly(3.4,5-tridodecyloxyphenylacetylene) (Poly5) and poly[3, 4, 5-tris((S)-3, 7-dimethyloctyloxy)phenylacetylene] (Poly6). PolyS and Poly6 are liquid crystalline with presumably a bilayer-type architecture in which the mesogens are arranged in an antiparallel overlapping interdigitated manner. Poly6 showed unusual thermal stereomutation in solution in a very narrow temperature range
    Original languageEnglish
    Pages (from-to)266-270
    Number of pages4
    JournalMacromolecular Rapid Communications
    Volume23
    Issue number4
    DOIs
    Publication statusPublished - 2002

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