Reconfiguring nanocomposite liquid crystal polymer films with visible light

A.W. Hauser, Danqing Liu, K.C. Bryson, R.C. Hayward, D.J. Broer

Research output: Contribution to journalArticleAcademicpeer-review

38 Citations (Scopus)
66 Downloads (Pure)

Abstract

Patterns of white light are projected on liquid crystal (LC) polymer films containing gold nanospheres (NS) or nanorods (NR) to induce out-of-plane buckling through a photothermal effect. Straightforward synthetic techniques are used to provide well-dispersed nanocomposite films, with NRs exhibiting self-alignment with the LC director. Using a combination of prepatterned director orientation and spatiotemporal variations in light intensity, these nanocomposite films can be reversibly configured into different 3D states. Fine control over shape is demonstrated through variations in size, shape, and intensity of the illuminated region. Switching time scales are found to be of order a few seconds or below, likely reflecting the intrinsic relaxation time of the LC materials.

Original languageEnglish
Pages (from-to)1575-1581
Number of pages7
JournalMacromolecules
Volume49
Issue number5
DOIs
Publication statusPublished - 9 Mar 2016

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