Pulsed corona oxidation of low NO and NO2 concentrations : semi-industrial tests and model simulations to illustrate the process

E.A. Filimonova, F.J.C.M. Beckers, R.W.J. Smulders, A.J.M. Pemen, W.F.L.M. Hoeben, E.J.M. Heesch, van

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Abstract

We present results of tests at semi-industrial scale accompanied by computer imulations, to illustrate the analysis of the reactor process and to test the applicability to traffic tunnel cleaning. The pollutant source is a diluted exhaust flow of a 15 kW Diesel engine. NOx input to the reactor is 30 ppm. The reactor is a 500 liter multiple-plate saw-blade structure fed by a 200 ns pulse source of 5 kW maximum average power. This source is a resonant charging system, pressurized spark gap and transmission line transformer. The computer model of removal process takes into account processes of chemical kinetics, diffusion outside and inside of streamer traces during multi-pulsed treatment and continued conversion in the inactive volume between reactor and point of gas sampling. Results show fair agreement between measured and simulated data of NO, NO2 and O3. HNO2, HNO3 production is shown as the completion of the process.
Original languageEnglish
Title of host publicationProceedings of the 63rd Gaseous Electronics Conference, 4-8 October 2010, Paris, France
PublisherGEC
PagesPR3-001-1/2
Publication statusPublished - 2010

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Oxidation
Electric sparks
Reaction kinetics
Diesel engines
Cleaning
Electric lines
Tunnels
Sampling
Gases

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Filimonova, E. A., Beckers, F. J. C. M., Smulders, R. W. J., Pemen, A. J. M., Hoeben, W. F. L. M., & Heesch, van, E. J. M. (2010). Pulsed corona oxidation of low NO and NO2 concentrations : semi-industrial tests and model simulations to illustrate the process. In Proceedings of the 63rd Gaseous Electronics Conference, 4-8 October 2010, Paris, France (pp. PR3-001-1/2). GEC.
Filimonova, E.A. ; Beckers, F.J.C.M. ; Smulders, R.W.J. ; Pemen, A.J.M. ; Hoeben, W.F.L.M. ; Heesch, van, E.J.M. / Pulsed corona oxidation of low NO and NO2 concentrations : semi-industrial tests and model simulations to illustrate the process. Proceedings of the 63rd Gaseous Electronics Conference, 4-8 October 2010, Paris, France. GEC, 2010. pp. PR3-001-1/2
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abstract = "We present results of tests at semi-industrial scale accompanied by computer imulations, to illustrate the analysis of the reactor process and to test the applicability to traffic tunnel cleaning. The pollutant source is a diluted exhaust flow of a 15 kW Diesel engine. NOx input to the reactor is 30 ppm. The reactor is a 500 liter multiple-plate saw-blade structure fed by a 200 ns pulse source of 5 kW maximum average power. This source is a resonant charging system, pressurized spark gap and transmission line transformer. The computer model of removal process takes into account processes of chemical kinetics, diffusion outside and inside of streamer traces during multi-pulsed treatment and continued conversion in the inactive volume between reactor and point of gas sampling. Results show fair agreement between measured and simulated data of NO, NO2 and O3. HNO2, HNO3 production is shown as the completion of the process.",
author = "E.A. Filimonova and F.J.C.M. Beckers and R.W.J. Smulders and A.J.M. Pemen and W.F.L.M. Hoeben and {Heesch, van}, E.J.M.",
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Filimonova, EA, Beckers, FJCM, Smulders, RWJ, Pemen, AJM, Hoeben, WFLM & Heesch, van, EJM 2010, Pulsed corona oxidation of low NO and NO2 concentrations : semi-industrial tests and model simulations to illustrate the process. in Proceedings of the 63rd Gaseous Electronics Conference, 4-8 October 2010, Paris, France. GEC, pp. PR3-001-1/2.

Pulsed corona oxidation of low NO and NO2 concentrations : semi-industrial tests and model simulations to illustrate the process. / Filimonova, E.A.; Beckers, F.J.C.M.; Smulders, R.W.J.; Pemen, A.J.M.; Hoeben, W.F.L.M.; Heesch, van, E.J.M.

Proceedings of the 63rd Gaseous Electronics Conference, 4-8 October 2010, Paris, France. GEC, 2010. p. PR3-001-1/2.

Research output: Chapter in Book/Report/Conference proceedingConference contributionAcademicpeer-review

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N2 - We present results of tests at semi-industrial scale accompanied by computer imulations, to illustrate the analysis of the reactor process and to test the applicability to traffic tunnel cleaning. The pollutant source is a diluted exhaust flow of a 15 kW Diesel engine. NOx input to the reactor is 30 ppm. The reactor is a 500 liter multiple-plate saw-blade structure fed by a 200 ns pulse source of 5 kW maximum average power. This source is a resonant charging system, pressurized spark gap and transmission line transformer. The computer model of removal process takes into account processes of chemical kinetics, diffusion outside and inside of streamer traces during multi-pulsed treatment and continued conversion in the inactive volume between reactor and point of gas sampling. Results show fair agreement between measured and simulated data of NO, NO2 and O3. HNO2, HNO3 production is shown as the completion of the process.

AB - We present results of tests at semi-industrial scale accompanied by computer imulations, to illustrate the analysis of the reactor process and to test the applicability to traffic tunnel cleaning. The pollutant source is a diluted exhaust flow of a 15 kW Diesel engine. NOx input to the reactor is 30 ppm. The reactor is a 500 liter multiple-plate saw-blade structure fed by a 200 ns pulse source of 5 kW maximum average power. This source is a resonant charging system, pressurized spark gap and transmission line transformer. The computer model of removal process takes into account processes of chemical kinetics, diffusion outside and inside of streamer traces during multi-pulsed treatment and continued conversion in the inactive volume between reactor and point of gas sampling. Results show fair agreement between measured and simulated data of NO, NO2 and O3. HNO2, HNO3 production is shown as the completion of the process.

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Filimonova EA, Beckers FJCM, Smulders RWJ, Pemen AJM, Hoeben WFLM, Heesch, van EJM. Pulsed corona oxidation of low NO and NO2 concentrations : semi-industrial tests and model simulations to illustrate the process. In Proceedings of the 63rd Gaseous Electronics Conference, 4-8 October 2010, Paris, France. GEC. 2010. p. PR3-001-1/2