Plastic deformation of glassy polymers : correlation between shear activation volume and entanglement density

J. Ho, L.E. Govaert, M. Utz

Research output: Chapter in Book/Report/Conference proceedingConference contributionAcademicpeer-review

2 Citations (Scopus)
2 Downloads (Pure)

Abstract

The shear activation volumes of miscible polystyrene-poly(2,6-dimethyl-1,4-phenylene oxide) (PS-PPO) blends at different PS-PPO ratios were determined experimentally by both plane strain and uniaxial compression at constant strain rates. We find that the shear activation volume is proportional to the entanglement density to the 0.6 power, and this correlation holds for the blend as well as for various pure glassy polymers. Since the shear activation volume is closely related to the size of the plastic shear zones, this correlation suggests that the cooperativity of the elementary processes of plastic deformation in glassy polymers scales with the entanglement density.
Original languageEnglish
Title of host publicationPolymer/metal interfaces and defect mediated phenomena in ordered polymers : symposia held December 2-6, 2002, Boston, Massachusetts, USA
EditorsE. Manias, G.G. Malliaras
Place of PublicationWarrendale
PublisherMaterials Research Society
Pages97-102
ISBN (Print)1-55899-671-0
Publication statusPublished - 2003
Eventconference; Polymer/metal interfaces and defect mediated phenomena in ordered polymers : symposia held December 2-6, 2002, Boston, Massachusetts, USA; 2002-12-02; 2002-12-06 -
Duration: 2 Dec 20026 Dec 2002

Publication series

NameMaterials Research Society symposium proceedings
Volume734

Conference

Conferenceconference; Polymer/metal interfaces and defect mediated phenomena in ordered polymers : symposia held December 2-6, 2002, Boston, Massachusetts, USA; 2002-12-02; 2002-12-06
Period2/12/026/12/02
OtherPolymer/metal interfaces and defect mediated phenomena in ordered polymers : symposia held December 2-6, 2002, Boston, Massachusetts, USA

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