On the CO2 and H2O chemisorption on hydrotalcite-based adsorbents for sorption-enhanced water-gas-shift processes.

K.T. Coenen; F. Gallucci; P.D. Cobden; H.A.J. van Dijk; E.J.M. Hensen; M. van Sint Annaland

On the CO2 and H2O chemisorption on hydrotalcite-based adsorbents for sorption-enhanced water-gas-shift processes.

K.T. Coenen
, F. Gallucci
, P.D. Cobden
, H.A.J. van Dijk
, E.J.M. Hensen
, M. van Sint Annaland

Research output: Contribution to conference › Poster

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Abstract

Thermogravimetric analysis (TGA) was used to study the adsorption phenomena of CO2 and H2O on a hydrotalcite-based adsorbent to be used for sorption-enhanced Water-Gas-Shift (SEWGS). The adsorption of CO2 and H2O and the interaction between the two can be described when considering the presence of at least three different sites (2 for CO2 and 1 for H2O) participating in the adsorption phenomena at elevated temperatures. The experiments confirm that the regeneration conditions are crucial for activating more sites for CO2 adsorption and are therefore the limiting factor for the cyclic working capacity of the adsorbent.

Original language	English
Publication status	Published - 14 Jun 2016
Event	24th International Symposium on Chemical Reaction Engineering (ISCRE 24) - Minneapolis, MN, United States Duration: 12 Jun 2016 → 15 Jun 2016 http://iscre.org/ISCRE24/

Conference

Conference	24th International Symposium on Chemical Reaction Engineering (ISCRE 24)
Abbreviated title	ISCRE 24
Country/Territory	United States
City	Minneapolis, MN
Period	12/06/16 → 15/06/16
Internet address	http://iscre.org/ISCRE24/

Keywords

Cyclic working capacity, CO2 sorption kinetics, Hydrotalcite

Cite this

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title = "On the CO2 and H2O chemisorption on hydrotalcite-based adsorbents for sorption-enhanced water-gas-shift processes.",

abstract = "Thermogravimetric analysis (TGA) was used to study the adsorption phenomena of CO2 and H2O on a hydrotalcite-based adsorbent to be used for sorption-enhanced Water-Gas-Shift (SEWGS). The adsorption of CO2 and H2O and the interaction between the two can be described when considering the presence of at least three different sites (2 for CO2 and 1 for H2O) participating in the adsorption phenomena at elevated temperatures. The experiments confirm that the regeneration conditions are crucial for activating more sites for CO2 adsorption and are therefore the limiting factor for the cyclic working capacity of the adsorbent.",

keywords = "Cyclic working capacity, CO2 sorption kinetics, Hydrotalcite",

author = "K.T. Coenen and F. Gallucci and P.D. Cobden and \{van Dijk\}, H.A.J. and E.J.M. Hensen and \{van Sint Annaland\}, M.",

year = "2016",

month = jun,

day = "14",

language = "English",

note = "24th International Symposium on Chemical Reaction Engineering (ISCRE 24), ISCRE 24 ; Conference date: 12-06-2016 Through 15-06-2016",

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TY - CONF

T1 - On the CO2 and H2O chemisorption on hydrotalcite-based adsorbents for sorption-enhanced water-gas-shift processes.

AU - Coenen, K.T.

AU - Gallucci, F.

AU - Cobden, P.D.

AU - van Dijk, H.A.J.

AU - Hensen, E.J.M.

AU - van Sint Annaland, M.

PY - 2016/6/14

Y1 - 2016/6/14

N2 - Thermogravimetric analysis (TGA) was used to study the adsorption phenomena of CO2 and H2O on a hydrotalcite-based adsorbent to be used for sorption-enhanced Water-Gas-Shift (SEWGS). The adsorption of CO2 and H2O and the interaction between the two can be described when considering the presence of at least three different sites (2 for CO2 and 1 for H2O) participating in the adsorption phenomena at elevated temperatures. The experiments confirm that the regeneration conditions are crucial for activating more sites for CO2 adsorption and are therefore the limiting factor for the cyclic working capacity of the adsorbent.

AB - Thermogravimetric analysis (TGA) was used to study the adsorption phenomena of CO2 and H2O on a hydrotalcite-based adsorbent to be used for sorption-enhanced Water-Gas-Shift (SEWGS). The adsorption of CO2 and H2O and the interaction between the two can be described when considering the presence of at least three different sites (2 for CO2 and 1 for H2O) participating in the adsorption phenomena at elevated temperatures. The experiments confirm that the regeneration conditions are crucial for activating more sites for CO2 adsorption and are therefore the limiting factor for the cyclic working capacity of the adsorbent.

KW - Cyclic working capacity, CO2 sorption kinetics, Hydrotalcite

M3 - Poster

T2 - 24th International Symposium on Chemical Reaction Engineering (ISCRE 24)

Y2 - 12 June 2016 through 15 June 2016

ER -

On the CO2 and H2O chemisorption on hydrotalcite-based adsorbents for sorption-enhanced water-gas-shift processes.

Abstract

Conference

Keywords

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