Noise spectroscopy of tunable nanoconstrictions: Molecule-free and molecule-modified

Volodymyr Handziuk, Ferdinand Gasparyan, Lode K.J. Vandamme, Maristella Coppola, Viktor Sydoruk, Mykhailo Petrychuk, Dirk Mayer, Svetlana Vitusevich

Research output: Contribution to journalArticleAcademicpeer-review

2 Citations (Scopus)

Abstract

Devices with metallic nanoconstrictions functionalized by organic molecules are promising candidates for the role of functional devices in molecular electronics. However, at the moment little is known about transport and noise properties of nanoconstriction devices of this kind. In this paper, transport properties of bare gold and molecule-containing tunable cross-section nanoconstrictions are studied using low-frequency noise spectroscopy. Normalized noise power spectral density (PSD) S I/I 2 dependencies are analyzed for a wide range of sample resistances R from 10 Ohm to 10 MOhm. The peculiarities and physical background of the flicker noise behavior in the low-bias regime are studied. It is shown that modification of the sample surface with benzene-1,4-dithiol molecules results in a decrease of the normalized flicker noise spectral density level in the ballistic regime of sample conductance. The characteristic power dependence of normalized noise PSD as a function of system resistance is revealed. Models describing noise behavior for bare gold and BDT modified samples are developed and compared with the experimental data for three transport regimes: diffusive, ballistic and tunneling. Parameters extracted from models by fitting are used for the characterization of nanoconstriction devices.

Original languageEnglish
Article number385704
Number of pages12
JournalNanotechnology
Volume29
Issue number38
DOIs
Publication statusPublished - 17 Jul 2018

Fingerprint

Power spectral density
Spectroscopy
Ballistics
Gold
Molecules
Molecular electronics
Spectral density
Benzene
Transport properties
N-((2,3-dihydro-1,4-benzodioxin-2-yl)methyl)-5-methoxy-1H-indole-3-ethanamine
dithiol

Keywords

  • nanoconstriction
  • noise spectroscopy
  • transport regimes

Cite this

Handziuk, V., Gasparyan, F., Vandamme, L. K. J., Coppola, M., Sydoruk, V., Petrychuk, M., ... Vitusevich, S. (2018). Noise spectroscopy of tunable nanoconstrictions: Molecule-free and molecule-modified. Nanotechnology, 29(38), [385704]. https://doi.org/10.1088/1361-6528/aad0b7
Handziuk, Volodymyr ; Gasparyan, Ferdinand ; Vandamme, Lode K.J. ; Coppola, Maristella ; Sydoruk, Viktor ; Petrychuk, Mykhailo ; Mayer, Dirk ; Vitusevich, Svetlana. / Noise spectroscopy of tunable nanoconstrictions : Molecule-free and molecule-modified. In: Nanotechnology. 2018 ; Vol. 29, No. 38.
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abstract = "Devices with metallic nanoconstrictions functionalized by organic molecules are promising candidates for the role of functional devices in molecular electronics. However, at the moment little is known about transport and noise properties of nanoconstriction devices of this kind. In this paper, transport properties of bare gold and molecule-containing tunable cross-section nanoconstrictions are studied using low-frequency noise spectroscopy. Normalized noise power spectral density (PSD) S I/I 2 dependencies are analyzed for a wide range of sample resistances R from 10 Ohm to 10 MOhm. The peculiarities and physical background of the flicker noise behavior in the low-bias regime are studied. It is shown that modification of the sample surface with benzene-1,4-dithiol molecules results in a decrease of the normalized flicker noise spectral density level in the ballistic regime of sample conductance. The characteristic power dependence of normalized noise PSD as a function of system resistance is revealed. Models describing noise behavior for bare gold and BDT modified samples are developed and compared with the experimental data for three transport regimes: diffusive, ballistic and tunneling. Parameters extracted from models by fitting are used for the characterization of nanoconstriction devices.",
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Handziuk, V, Gasparyan, F, Vandamme, LKJ, Coppola, M, Sydoruk, V, Petrychuk, M, Mayer, D & Vitusevich, S 2018, 'Noise spectroscopy of tunable nanoconstrictions: Molecule-free and molecule-modified', Nanotechnology, vol. 29, no. 38, 385704. https://doi.org/10.1088/1361-6528/aad0b7

Noise spectroscopy of tunable nanoconstrictions : Molecule-free and molecule-modified. / Handziuk, Volodymyr; Gasparyan, Ferdinand; Vandamme, Lode K.J.; Coppola, Maristella; Sydoruk, Viktor; Petrychuk, Mykhailo; Mayer, Dirk; Vitusevich, Svetlana.

In: Nanotechnology, Vol. 29, No. 38, 385704, 17.07.2018.

Research output: Contribution to journalArticleAcademicpeer-review

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AU - Handziuk, Volodymyr

AU - Gasparyan, Ferdinand

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AU - Coppola, Maristella

AU - Sydoruk, Viktor

AU - Petrychuk, Mykhailo

AU - Mayer, Dirk

AU - Vitusevich, Svetlana

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