Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions

M.A. Tas; R.M. van Hardeveld; E.M. Veldhuizen, van; R.A. Santen, van

Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions

M.A. Tas, R.M. van Hardeveld, E.M. Veldhuizen, van, R.A. Santen, van

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

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Abstract

A model is developed to describe the transfer of vibrational energy from excited gas molecules to a heterogeneous surface or to heating of the gas. Diffusion of excited species is included in the model. The model is used to compute the maximum possible energy efficiency of a plasma-induced catalytic reaction, which is driven by vibrationally excited molecules. The computational results of the model are correlated to experimental data on quenching rates and the relevant parameters of the self-sustained discharge. It is con cluded that the mechanism of plasma-induced catalysis with vibrationally excited molecules is highly unlikely.

Original language	English
Title of host publication	Proceedings of the 12th International Symposium on Plasma Chemistry (ISPC-12) 21-25 August 1995 Minneapolis, Minnesota, USA
Editors	J.V. Heberlein, D.W. Ernie, J.T. Roberts
Place of Publication	Minneapolis, Minn.
Publisher	American Physical Society
Pages	481-486
Number of pages	6
ISBN (Print)	1-88797-600-0
Publication status	Published - 1995
Event	12th International Symposium on Plasma Chemistry (ISPC 12), August 21-25, 1995, Minneapolis, MN, USA - Minneapolis, MN, United States Duration: 21 Aug 1995 → 25 Aug 1995

Conference

Conference	12th International Symposium on Plasma Chemistry (ISPC 12), August 21-25, 1995, Minneapolis, MN, USA
Abbreviated title	ISPC 12
Country/Territory	United States
City	Minneapolis, MN
Period	21/08/95 → 25/08/95
Other	Proc. 12th International Symposium on Plasma Chemistry, Minneapolis

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Tas, M. A., van Hardeveld, R. M., Veldhuizen, van, E. M., & Santen, van, R. A. (1995). Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions. In J. V. Heberlein, D. W. Ernie, & J. T. Roberts (Eds.), Proceedings of the 12th International Symposium on Plasma Chemistry (ISPC-12) 21-25 August 1995 Minneapolis, Minnesota, USA (pp. 481-486). American Physical Society.

Tas, M.A. ; van Hardeveld, R.M. ; Veldhuizen, van, E.M. et al. / Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions. Proceedings of the 12th International Symposium on Plasma Chemistry (ISPC-12) 21-25 August 1995 Minneapolis, Minnesota, USA. editor / J.V. Heberlein ; D.W. Ernie ; J.T. Roberts. Minneapolis, Minn. : American Physical Society, 1995. pp. 481-486

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title = "Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions",

abstract = "A model is developed to describe the transfer of vibrational energy from excited gas molecules to a heterogeneous surface or to heating of the gas. Diffusion of excited species is included in the model. The model is used to compute the maximum possible energy efficiency of a plasma-induced catalytic reaction, which is driven by vibrationally excited molecules. The computational results of the model are correlated to experimental data on quenching rates and the relevant parameters of the self-sustained discharge. It is con cluded that the mechanism of plasma-induced catalysis with vibrationally excited molecules is highly unlikely.",

author = "M.A. Tas and {van Hardeveld}, R.M. and {Veldhuizen, van}, E.M. and {Santen, van}, R.A.",

year = "1995",

language = "English",

isbn = "1-88797-600-0",

pages = "481--486",

editor = "J.V. Heberlein and D.W. Ernie and J.T. Roberts",

booktitle = "Proceedings of the 12th International Symposium on Plasma Chemistry (ISPC-12) 21-25 August 1995 Minneapolis, Minnesota, USA",

publisher = "American Physical Society",

address = "United States",

note = "12th International Symposium on Plasma Chemistry (ISPC 12), August 21-25, 1995, Minneapolis, MN, USA, ISPC 12 ; Conference date: 21-08-1995 Through 25-08-1995",

}

Tas, MA, van Hardeveld, RM, Veldhuizen, van, EM & Santen, van, RA 1995, Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions. in JV Heberlein, DW Ernie & JT Roberts (eds), Proceedings of the 12th International Symposium on Plasma Chemistry (ISPC-12) 21-25 August 1995 Minneapolis, Minnesota, USA. American Physical Society, Minneapolis, Minn., pp. 481-486, 12th International Symposium on Plasma Chemistry (ISPC 12), August 21-25, 1995, Minneapolis, MN, USA, Minneapolis, MN, United States, 21/08/95.

Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions. / Tas, M.A.; van Hardeveld, R.M.; Veldhuizen, van, E.M. et al.
Proceedings of the 12th International Symposium on Plasma Chemistry (ISPC-12) 21-25 August 1995 Minneapolis, Minnesota, USA. ed. / J.V. Heberlein; D.W. Ernie; J.T. Roberts. Minneapolis, Minn.: American Physical Society, 1995. p. 481-486.

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › Academic › peer-review

TY - GEN

T1 - Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions

AU - Tas, M.A.

AU - van Hardeveld, R.M.

AU - Veldhuizen, van, E.M.

AU - Santen, van, R.A.

PY - 1995

Y1 - 1995

N2 - A model is developed to describe the transfer of vibrational energy from excited gas molecules to a heterogeneous surface or to heating of the gas. Diffusion of excited species is included in the model. The model is used to compute the maximum possible energy efficiency of a plasma-induced catalytic reaction, which is driven by vibrationally excited molecules. The computational results of the model are correlated to experimental data on quenching rates and the relevant parameters of the self-sustained discharge. It is con cluded that the mechanism of plasma-induced catalysis with vibrationally excited molecules is highly unlikely.

AB - A model is developed to describe the transfer of vibrational energy from excited gas molecules to a heterogeneous surface or to heating of the gas. Diffusion of excited species is included in the model. The model is used to compute the maximum possible energy efficiency of a plasma-induced catalytic reaction, which is driven by vibrationally excited molecules. The computational results of the model are correlated to experimental data on quenching rates and the relevant parameters of the self-sustained discharge. It is con cluded that the mechanism of plasma-induced catalysis with vibrationally excited molecules is highly unlikely.

M3 - Conference contribution

SN - 1-88797-600-0

SP - 481

EP - 486

BT - Proceedings of the 12th International Symposium on Plasma Chemistry (ISPC-12) 21-25 August 1995 Minneapolis, Minnesota, USA

A2 - Heberlein, J.V.

A2 - Ernie, D.W.

A2 - Roberts, J.T.

PB - American Physical Society

CY - Minneapolis, Minn.

T2 - 12th International Symposium on Plasma Chemistry (ISPC 12), August 21-25, 1995, Minneapolis, MN, USA

Y2 - 21 August 1995 through 25 August 1995

ER -

Tas MA, van Hardeveld RM, Veldhuizen, van EM, Santen, van RA. Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions. In Heberlein JV, Ernie DW, Roberts JT, editors, Proceedings of the 12th International Symposium on Plasma Chemistry (ISPC-12) 21-25 August 1995 Minneapolis, Minnesota, USA. Minneapolis, Minn.: American Physical Society. 1995. p. 481-486

Modeling of the reactivity of vibrationally excited molecules in a corona plasma for catalytic reactions

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