Demonstration of a packed bed membrane reactor for the oxidative dehydrogenation of propane

Ž.S. Kotanjac; M. Sint Annaland, van; J.A.M. Kuipers

doi:10.1016/j.ces.2010.08.037

Demonstration of a packed bed membrane reactor for the oxidative dehydrogenation of propane

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Abstract

An experimental demonstration of the oxidative dehydrogenation of propane (ODHP) in a lab-scale packed bed membrane reactor has been performed. Experiments were carried out with both premixed and distributed oxygen feed over a Ga₂O₃/MoO₃ catalyst and compared, and the influence of the gas composition, flow rate and the extent of dilution was investigated. The experimental results were found to compare very well with detailed reactor simulations. The results revealed that, in comparison with conventional reactor concepts for the ODHP (fixed bed with premixed reactants feed), a significantly higher propylene yield can be achieved at higher propane conversions in a packed bed membrane reactor. © 2010 Elsevier Ltd.

Original language	English
Pages (from-to)	6029-6035
Journal	Chemical Engineering Science
Volume	65
Issue number	22
DOIs	https://doi.org/10.1016/j.ces.2010.08.037
Publication status	Published - 2010

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title = "Demonstration of a packed bed membrane reactor for the oxidative dehydrogenation of propane",

abstract = "An experimental demonstration of the oxidative dehydrogenation of propane (ODHP) in a lab-scale packed bed membrane reactor has been performed. Experiments were carried out with both premixed and distributed oxygen feed over a Ga2O3/MoO3 catalyst and compared, and the influence of the gas composition, flow rate and the extent of dilution was investigated. The experimental results were found to compare very well with detailed reactor simulations. The results revealed that, in comparison with conventional reactor concepts for the ODHP (fixed bed with premixed reactants feed), a significantly higher propylene yield can be achieved at higher propane conversions in a packed bed membrane reactor. {\textcopyright} 2010 Elsevier Ltd.",

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T1 - Demonstration of a packed bed membrane reactor for the oxidative dehydrogenation of propane

AU - Kotanjac, Ž.S.

AU - Sint Annaland, van, M.

AU - Kuipers, J.A.M.

PY - 2010

Y1 - 2010

N2 - An experimental demonstration of the oxidative dehydrogenation of propane (ODHP) in a lab-scale packed bed membrane reactor has been performed. Experiments were carried out with both premixed and distributed oxygen feed over a Ga2O3/MoO3 catalyst and compared, and the influence of the gas composition, flow rate and the extent of dilution was investigated. The experimental results were found to compare very well with detailed reactor simulations. The results revealed that, in comparison with conventional reactor concepts for the ODHP (fixed bed with premixed reactants feed), a significantly higher propylene yield can be achieved at higher propane conversions in a packed bed membrane reactor. © 2010 Elsevier Ltd.

AB - An experimental demonstration of the oxidative dehydrogenation of propane (ODHP) in a lab-scale packed bed membrane reactor has been performed. Experiments were carried out with both premixed and distributed oxygen feed over a Ga2O3/MoO3 catalyst and compared, and the influence of the gas composition, flow rate and the extent of dilution was investigated. The experimental results were found to compare very well with detailed reactor simulations. The results revealed that, in comparison with conventional reactor concepts for the ODHP (fixed bed with premixed reactants feed), a significantly higher propylene yield can be achieved at higher propane conversions in a packed bed membrane reactor. © 2010 Elsevier Ltd.

U2 - 10.1016/j.ces.2010.08.037

DO - 10.1016/j.ces.2010.08.037

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VL - 65

SP - 6029

EP - 6035

JO - Chemical Engineering Science

JF - Chemical Engineering Science

IS - 22

ER -

Demonstration of a packed bed membrane reactor for the oxidative dehydrogenation of propane

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